Enantioselective supercritical fluid chromatography-tandem mass spectrometry method for simultaneous estimation of risperidone and its 9-hydroxyl metabolites in rat plasma

Bioanalysis. 2017 Nov;9(22):1739-1750. doi: 10.4155/bio-2017-0168. Epub 2017 Nov 9.

Abstract

Aim: Objective of the current work was to develop a 'green chemistry' compliant selective and sensitive supercritical fluid chromatography-tandem mass spectrometry method for simultaneous estimation of risperidone (RIS) and its chiral metabolites in rat plasma. Methodology & results: Agilent 1260 Infinity analytical supercritical fluid chromatography system resolved RIS and its chiral metabolites within runtime of 6 min using a gradient chromatography method. Using a simple protein precipitation sample preparation followed by mass spectrometric detection achieved a sensitivity of 0.92 nM (lower limit of quantification). With linearity over four log units (0.91-7500 nM), the method was found to be selective, accurate, precise and robust.

Conclusion: The method was validated and was successfully applied for simultaneous estimation of RIS and 9-hydroxyrisperidone metabolites (R & S individually) after intravenous and per oral administration to rats.

Keywords: 9-hydroxyrisperidone; SFC–MS/MS; chiral metabolites; pharmacokinetics; risperidone; supercritical fluid chromatography.

MeSH terms

  • Animals
  • Chromatography, Supercritical Fluid / methods*
  • Half-Life
  • Limit of Detection
  • Male
  • Rats
  • Rats, Sprague-Dawley
  • Reproducibility of Results
  • Risperidone / blood*
  • Risperidone / metabolism
  • Risperidone / pharmacokinetics
  • Stereoisomerism
  • Tandem Mass Spectrometry / methods*

Substances

  • Risperidone