Formulation, evaluation and bioactive potential of Xylaria primorskensis terpenoid nanoparticles from its major compound xylaranic acid

Sci Rep. 2018 Jan 29;8(1):1740. doi: 10.1038/s41598-018-20237-z.

Abstract

In recent years, fungi have been shown to produce a plethora of new bioactive secondary metabolites of interest, as new lead structures for medicinal and other pharmacological applications. The present investigation was carried out to study the pharmacological properties of a potent and major bioactive compound: xylaranic acid, which was obtained from Xylaria primorskensis (X. primorskensis) terpenoids in terms of antibacterial activity, antioxidant potential against DPPH & H2O2 radicals and anticancer activity against human lung cancer cells. Due to terpenoid nature, low water solubility and wretched bioavailability, its pharmacological use is limited. To overcome these drawbacks, a novel xylaranic acid silver nanoparticle system (AgNPs) is developed. In addition to improving its solubility and bioavailability, other advantageous pharmacological properties has been evaluated. Furthermore, enhanced anticancer activity of xylaranic acid and its AgNPs due to induced apoptosis were also confirmed by determining the expression levels of apoptosis regulatory genes p53, bcl-2 and caspase-3 via qRT PCR method. This is the first study developing the novel xylaranic acid silver nanoparticle system and enlightening its therapeutic significance with its improved physico-chemical properties and augmented bioactive potential.

MeSH terms

  • A549 Cells
  • Anti-Bacterial Agents / isolation & purification
  • Anti-Bacterial Agents / pharmacokinetics
  • Anti-Bacterial Agents / pharmacology*
  • Antineoplastic Agents / isolation & purification
  • Antineoplastic Agents / pharmacokinetics
  • Antineoplastic Agents / pharmacology*
  • Antioxidants / isolation & purification
  • Antioxidants / pharmacokinetics
  • Antioxidants / pharmacology*
  • Apoptosis
  • Apoptosis Regulatory Proteins / biosynthesis
  • Apoptosis Regulatory Proteins / genetics
  • Cell Survival / drug effects
  • Drug Carriers*
  • Epithelial Cells / drug effects
  • Epithelial Cells / physiology
  • Free Radical Scavengers / pharmacology
  • Gene Expression Profiling
  • Humans
  • Inhibitory Concentration 50
  • Metal Nanoparticles*
  • Microbial Sensitivity Tests
  • Silver
  • Solubility
  • Terpenes / isolation & purification
  • Terpenes / pharmacokinetics
  • Terpenes / pharmacology*
  • Xylariales / chemistry*
  • Xylariales / classification
  • Xylariales / genetics
  • Xylariales / isolation & purification

Substances

  • Anti-Bacterial Agents
  • Antineoplastic Agents
  • Antioxidants
  • Apoptosis Regulatory Proteins
  • Drug Carriers
  • Free Radical Scavengers
  • Terpenes
  • Silver