A facile consensus ranking approach enhances virtual screening robustness and identifies a cell-active DYRK1α inhibitor

Future Med Chem. 2018 Oct;10(20):2411-2430. doi: 10.4155/fmc-2018-0198. Epub 2018 Oct 16.

Abstract

Background: Virtual screening is vital for contemporary drug discovery but striking performance fluctuations are commonly encountered, thus hampering error-free use. Results and Methodology: A conceptual framework is suggested for combining screening algorithms characterized by orthogonality (docking-scoring calculations, 3D shape similarity, 2D fingerprint similarity) into a simple, efficient and expansible python-based consensus ranking scheme. An original experimental dataset is created for comparing individual screening methods versus the novel approach. Its utilization leads to identification and phosphoproteomic evaluation of a cell-active DYRK1α inhibitor.

Conclusion: Consensus ranking considerably stabilizes screening performance at reasonable computational cost, whereas individual screens are heavily dependent on calculation settings. Results indicate that the novel approach, currently available as a free online tool, is highly suitable for prospective screening by nonexperts.

Keywords: CREB1; NCI diversity set-II; NSC379099; analysis of residuals; docking-scoring calculations; fingerprint similarity; p53; phosphoproteomics; screening enrichment; shape-based similarity.

Publication types

  • Research Support, N.I.H., Extramural

MeSH terms

  • Algorithms
  • Cell Line
  • Cell Survival / drug effects
  • Consensus
  • Databases, Pharmaceutical
  • Drug Discovery / methods
  • Drug Evaluation, Preclinical / methods
  • Dyrk Kinases
  • Humans
  • Molecular Docking Simulation / methods
  • Prospective Studies
  • Protein Kinase Inhibitors / chemistry*
  • Protein Kinase Inhibitors / pharmacology
  • Protein Serine-Threonine Kinases / antagonists & inhibitors*
  • Protein-Tyrosine Kinases / antagonists & inhibitors*

Substances

  • Protein Kinase Inhibitors
  • Protein-Tyrosine Kinases
  • Protein Serine-Threonine Kinases