Novel imiquimod nanovesicles for topical vaccination

Colloids Surf B Biointerfaces. 2019 Feb 1:174:536-543. doi: 10.1016/j.colsurfb.2018.11.031. Epub 2018 Nov 15.

Abstract

Development of needle and pain free noninvasive immunization procedures is a top priority for public health agencies. In this work the topical adjuvant activity of the immunomodulator imiquimod (IMQ) carried by ultradeformable archaeosomes (UDA2) (nanovesicles containing sn-2,3 ether linked phytanyl saturated archaeolipids) was surveyed and compared with that of ultradeformable liposomes lacking archaeolipids (UDL2) and free IMQ, using the model antigen ovalbumin and a seasonal influenza vaccine in Balb/c mice. UDA2 (250 ± 94 nm, -26 ± 4 mV Z potential) induced higher IMQ accumulation in human skin and higher production of TNF-α and IL-6 by macrophages and keratinocytes than free IMQ and UDL2. Mixed with ovalbumin, UDA2 was more efficient at generating cellular response, as measured by an increase in serum IgG2a and INF-γ production by splenocytes, compared with free IMQ and UDL2. Moreover, mixed with a seasonal influenza vaccine UDA2 produced same IgG titers and IgG2a/IgG1 isotypes ratio (≈1) than the subcutaneously administered influenza vaccine. Topical UDA2 however, induced highest stimulation index and INF-γ levels by splenocytes. UDA2 might be a promising adjuvant for topical immunization, since it produced cell-biased systemic response with ≈ 13-fold lower IMQ dose than the delivered as the commercial IMQ cream, Aldara.

Keywords: Archaeolipids; Cellular response; Immunomodulator; Influenza vaccine.

MeSH terms

  • Adjuvants, Immunologic / administration & dosage
  • Administration, Topical
  • Animals
  • Cell Proliferation
  • Cells, Cultured
  • Cytokines / metabolism
  • Halorubrum / immunology*
  • Humans
  • Imiquimod / administration & dosage*
  • Imiquimod / immunology
  • Keratinocytes / cytology
  • Keratinocytes / drug effects
  • Keratinocytes / immunology*
  • Liposomes
  • Macrophages / cytology
  • Macrophages / drug effects
  • Macrophages / immunology*
  • Male
  • Mice
  • Mice, Inbred BALB C
  • Nanoparticles / administration & dosage*
  • Nanoparticles / chemistry
  • Ovalbumin / immunology
  • Skin / cytology
  • Skin / drug effects
  • Skin / immunology*
  • Vaccination / methods*

Substances

  • Adjuvants, Immunologic
  • Cytokines
  • Liposomes
  • Ovalbumin
  • Imiquimod