In-situ Chemiluminescence-Driven Reversible Addition-Fragmentation Chain-Transfer Photopolymerization

Angew Chem Int Ed Engl. 2019 Aug 19;58(34):11826-11829. doi: 10.1002/anie.201905317. Epub 2019 Jul 25.

Abstract

The power of chemical light generation (chemiluminescence) is used to drive polymerization reactions. A biphasic reaction is developed such that light-generating reactions are confined to the organic phase and photopolymerization occurs in the aqueous phase. Well-defined RAFT-capped polymers are synthesized and the kinetics are shown to be dictated by light generation.

Keywords: Chemiluminescence; Kinetics; Photochemistry; Photopolymerization; Reversible addition-fragmentation chain transfer polymerization.