Repurposing Approved Drugs as Inhibitors of Kv7.1 and Nav1.8 to Treat Pitt Hopkins Syndrome

Pharm Res. 2019 Jul 22;36(9):137. doi: 10.1007/s11095-019-2671-y.

Abstract

Purpose: Pitt Hopkins Syndrome (PTHS) is a rare genetic disorder caused by mutations of a specific gene, transcription factor 4 (TCF4), located on chromosome 18. PTHS results in individuals that have moderate to severe intellectual disability, with most exhibiting psychomotor delay. PTHS also exhibits features of autistic spectrum disorders, which are characterized by the impaired ability to communicate and socialize. PTHS is comorbid with a higher prevalence of epileptic seizures which can be present from birth or which commonly develop in childhood. Attenuated or absent TCF4 expression results in increased translation of peripheral ion channels Kv7.1 and Nav1.8 which triggers an increase in after-hyperpolarization and altered firing properties.

Methods: We now describe a high throughput screen (HTS) of 1280 approved drugs and machine learning models developed from this data. The ion channels were expressed in either CHO (KV7.1) or HEK293 (Nav1.8) cells and the HTS used either 86Rb+ efflux (KV7.1) or a FLIPR assay (Nav1.8).

Results: The HTS delivered 55 inhibitors of Kv7.1 (4.2% hit rate) and 93 inhibitors of Nav1.8 (7.2% hit rate) at a screening concentration of 10 μM. These datasets also enabled us to generate and validate Bayesian machine learning models for these ion channels. We also describe a structure activity relationship for several dihydropyridine compounds as inhibitors of Nav1.8.

Conclusions: This work could lead to the potential repurposing of nicardipine or other dihydropyridine calcium channel antagonists as potential treatments for PTHS acting via Nav1.8, as there are currently no approved treatments for this rare disorder.

Keywords: Kv7.1; Nav1.8; Pitt Hopkins syndrome; high throughput screen; repurposing.

MeSH terms

  • Animals
  • Bayes Theorem
  • CHO Cells
  • Cricetulus
  • Dihydropyridines / chemistry
  • Dihydropyridines / pharmacology*
  • Drug Repositioning / methods*
  • Facies
  • HEK293 Cells
  • Humans
  • Hyperventilation / drug therapy*
  • Intellectual Disability / drug therapy*
  • KCNQ1 Potassium Channel / antagonists & inhibitors*
  • KCNQ1 Potassium Channel / metabolism
  • Machine Learning
  • NAV1.8 Voltage-Gated Sodium Channel / metabolism*
  • Potassium Channel Blockers / chemistry
  • Potassium Channel Blockers / pharmacology*
  • Small Molecule Libraries / chemistry
  • Sodium Channel Blockers / chemistry
  • Sodium Channel Blockers / pharmacology*
  • Structure-Activity Relationship
  • Voltage-Gated Sodium Channel Blockers / chemistry
  • Voltage-Gated Sodium Channel Blockers / pharmacology*

Substances

  • Dihydropyridines
  • KCNQ1 Potassium Channel
  • NAV1.8 Voltage-Gated Sodium Channel
  • Potassium Channel Blockers
  • Small Molecule Libraries
  • Sodium Channel Blockers
  • Voltage-Gated Sodium Channel Blockers

Supplementary concepts

  • Pitt-Hopkins syndrome