Anti-malarial ozonides OZ439 and OZ609 tested at clinically relevant compound exposure parameters in a novel ring-stage survival assay

Malar J. 2019 Dec 18;18(1):427. doi: 10.1186/s12936-019-3056-8.

Abstract

Background: Drug efficacy against kelch 13 mutant malaria parasites can be determined in vitro with the ring-stage survival assay (RSA). The conventional assay protocol reflects the exposure profile of dihydroartemisinin.

Methods: Taking into account that other anti-malarial peroxides, such as the synthetic ozonides OZ439 (artefenomel) and OZ609, have different pharmacokinetics, the RSA was adjusted to the concentration-time profile of these ozonides in humans and a novel, semi-automated readout was introduced.

Results: When tested at clinically relevant parameters, it was shown that OZ439 and OZ609 are active against the Plasmodium falciparum clinical isolate Cam3.IR539T.

Conclusion: If the in vitro RSA does indeed predict the potency of compounds against parasites with increased tolerance to artemisinin and its derivatives, then the herein presented data suggest that following drug-pulses of at least 48 h, OZ439 and OZ609 will be highly potent against kelch 13 mutant isolates, such as P. falciparum Cam3.IR539T.

Keywords: Artemisinins; Cam3.IR539T; Malaria; Ozonides; Plasmodium falciparum; RSA; kelch 13.

MeSH terms

  • Adamantane / analogs & derivatives*
  • Adamantane / pharmacology
  • Antimalarials / pharmacology*
  • Dose-Response Relationship, Drug
  • Humans
  • Malaria, Falciparum / drug therapy
  • Peroxides / pharmacology*
  • Plasmodium falciparum / drug effects*

Substances

  • Antimalarials
  • Peroxides
  • Adamantane
  • artefenomel