A novel class of small molecule inhibitors with radioprotective properties

Eur J Med Chem. 2020 Feb 1:187:111606. doi: 10.1016/j.ejmech.2019.111606. Epub 2020 Jan 1.

Abstract

The goal of this study was to develop novel radioprotective agents targeting the intrinsic apoptotic pathway and thus decreasing the radiation-induced damage. For that purpose, we designed, synthesized and analyzed ten new compounds based on the 1-(4-(2-hydroxyethyl)piperazin-1-yl)-3-phenoxypropan-2-ol leading structure. The cytotoxicity of the newly synthesized substances was tested in vitro on cell lines derived from different progenitor cells by WST-1 proliferation assay. MTT test was utilized to assess half-maximal inhibitory concentrations and maximum tolerated concentrations of novel compounds in A-549 cells. Screening for radioprotective properties was performed using flow-cytometry in MOLT-4 cells exposed to 60Co ionizing gamma radiation. Selected candidates underwent in vivo testing in C57Bl/6 J mice having a positive impact on their immunological status. In summary, we report here promising compounds with radioprotective effect in vivo.

Keywords: 1-(2-hydroxyethyl)piperazine derivative; In vitro; Ionizing radiation; Mice; Radioprotection; Synthesis.

MeSH terms

  • Animals
  • Apoptosis / drug effects
  • Cell Line, Tumor
  • Cell Proliferation / drug effects
  • Dose-Response Relationship, Drug
  • Humans
  • Mice
  • Mice, Inbred C57BL
  • Molecular Docking Simulation
  • Molecular Structure
  • Propanols / chemical synthesis
  • Propanols / chemistry
  • Propanols / pharmacology*
  • Radiation-Protective Agents / chemical synthesis
  • Radiation-Protective Agents / chemistry
  • Radiation-Protective Agents / pharmacology*
  • Small Molecule Libraries / chemical synthesis
  • Small Molecule Libraries / chemistry
  • Small Molecule Libraries / pharmacology*
  • Structure-Activity Relationship

Substances

  • Propanols
  • Radiation-Protective Agents
  • Small Molecule Libraries