Photoacoustic 3-D imaging of polycrystalline microstructure improved with transverse acoustic waves

Théo Thréard; Elton de Lima Savi; Sergey Avanesyan; Nikolay Chigarev; Zilong Hua; Vincent Tournat; Vitalyi E Gusev; David H Hurley; Samuel Raetz

doi:10.1016/j.pacs.2021.100286

Photoacoustic 3-D imaging of polycrystalline microstructure improved with transverse acoustic waves

Photoacoustics. 2021 Aug 2:23:100286. doi: 10.1016/j.pacs.2021.100286. eCollection 2021 Sep.

Authors

Théo Thréard¹, Elton de Lima Savi¹, Sergey Avanesyan², Nikolay Chigarev¹, Zilong Hua³, Vincent Tournat¹, Vitalyi E Gusev¹, David H Hurley³, Samuel Raetz¹

Affiliations

¹ Laboratoire d'Acoustique de l'Université du Mans (LAUM), UMR 6613, Institut d'Acoustique - Graduate School (IA-GS), CNRS, Le Mans Université, France.
² Departement of Life and Physical Sciences, Fisk University, Nashville, USA.
³ Idaho National Laboratory, P.O. Box 1625, Idaho Falls, ID 83415, USA.

Abstract

Non-invasive fast imaging of grain microstructure of polycrystalline ceria with sub-micrometric spatial resolution is performed via time-domain Brillouin scattering. The propagation of a nanoacoustic pulse is monitored down to 8 μm deep in a 30 × 30 μm² area. Grains boundaries are reconstructed in three-dimensions via a two-step processing method, relying on the wavelet synchro-squeezed transform and the alphashape algorithm. Imaging contrast is improved by taking advantage of stronger sensitivity to anisotropy of transverse acoustic waves, compared with longitudinal waves. Utilization of transverse waves in the image processing reveals additional boundaries, confirmed by an electron backscattering diffraction pattern but not discerned using longitudinal waves. A buried inclined interface between differently oriented grains is identified by monitoring changes in amplitude (phase) of the portion of the signal associated with transverse (longitudinal) waves. Estimates of the inclination angle of this interface prove the sensitivity of our laser ultrasonic method to image inclined boundaries.

Keywords: 3-D imaging; Asynchronous optical sampling; Inclined grain boundary; Picosecond acoustic interferometry; Polycrystalline material; Time-domain Brillouin scattering (TDBS); Transverse-elastic-waves enhanced contrast; Wavelet synchro-squeezed transform.