Pharmacokinetics and metabolic disposition of a potent and selective kynurenine monooxygenase inhibitor, CHDI-340246, in laboratory animals

Xenobiotica. 2021 Oct;51(10):1155-1180. doi: 10.1080/00498254.2021.1977868. Epub 2021 Sep 15.

Abstract

The disposition of a novel kynurenine monooxygenase inhibitor, CHDI-340246, was investigated in vitro and in animals.In vitro, there was minimal metabolic turnover of CHDI-340246 in all species. The protein binding was higher in human plasma (99.7%) relative to other species.In all species, blood clearance was low (<20% of liver blood flow) and volume of distribution was small (<0.5 L/kg). The terminal half-life was longer in monkeys (9 hr) than in mice, rats, or dogs (1-2 hr). CHDI-340246 was orally bioavailable (>60%) in all species.In rats, [14C]CHDI-340246 showed wide distribution of radioactivity in all tissues except brain and testes. In rats, the parent drug was the major circulating moiety with minor amounts of a sulphate conjugate of an O-dealkylated metabolite. The elimination occurred via the urinary route and to a lesser extent by biliary route, but mostly as metabolites. In cynomolgus monkeys, the parent drug predominated in plasma with only trace amounts of metabolites detected.Acyl glucuronide conjugate of CHDI-340246 was not detected in plasma of rats or monkeys.Overall, the ADME profile of CHDI-340246 was favourable in rats and monkeys for potential evaluation of KMO inhibition in humans.

Keywords: ADME; CHDI-340246; KMO inhibitor; cynomolgus monkey; metabolite identification; pharmacokinetics; radiometabolite profiling; rat; tissue distribution.

MeSH terms

  • Animals
  • Animals, Laboratory
  • Dogs
  • Kynurenine*
  • Mice
  • Mixed Function Oxygenases
  • Pyrimidines*
  • Rats
  • Species Specificity

Substances

  • CHDI-340246
  • Pyrimidines
  • Kynurenine
  • Mixed Function Oxygenases