Development and validation of a novel evaporation setup-assisted TLC method with fluorescence detection for determination of flibanserin in pharmaceutical and biological samples

J Chromatogr B Analyt Technol Biomed Life Sci. 2022 Apr 15:1195:123204. doi: 10.1016/j.jchromb.2022.123204. Epub 2022 Mar 2.

Abstract

A specific and sensitive thin layer chromatographic method coupled with fluorescence detection for determination of flibanserin (FLN) that treats woman hypoactive sexual desire disorder was developed. The proposed method depends on the enhancement of FLN native fluorescence intensity via the exposure of the developed TLC plate to concentrated hydrochloric acid vapors. Herein, an evaporation setup needed for HCl vapors exposure step was designed for the first time to ensure a uniform distribution of the vapors throughout the developed bands on the plate. Chloroform: methanol (9.5: 0.5, v/v) was the optimum mobile phase that gave a compact band (Rf= 0.44 ± 0.02) using TLC aluminium plates precoated with silica gel G 60F254 as a stationary phase. After exposure of the developed TLC plate to HCl vapors, the FLN bands emission intensities were measured after excitation at 275 nm. Conferring ICH guidelines, the linearity range was 20.0 - 1500.0 ng/band with a good linear relationship (r= 0.9998). Detection and quantitation limits were 5.12 and 15.50 ng/band, respectively. Also, the method was validated for accuracy, precision, robustness, specificity and selectivity. Statistical analysis verified the suitability of the proposed method for estimation of FLN in tablets and in human plasma with acceptable recoveries (98.07-101.45%).

Keywords: Evaporation setup; Flibanserin; Fluorescence detection; Plasma; Tablets; Thin layer chromatography.

MeSH terms

  • Benzimidazoles* / analysis
  • Benzimidazoles* / blood
  • Benzimidazoles* / chemistry
  • Chromatography, Thin Layer / methods*
  • Humans
  • Limit of Detection
  • Linear Models
  • Reproducibility of Results
  • Spectrometry, Fluorescence / methods*
  • Tablets

Substances

  • Benzimidazoles
  • Tablets
  • flibanserin