The Phospholipase Activity of Ammodytoxin, a Prototype Snake Venom β-Neurotoxin, Is Not Obligatory for Cell Internalisation and Translocation to Mitochondria

Toxins (Basel). 2022 May 28;14(6):375. doi: 10.3390/toxins14060375.

Abstract

β-Neurotoxins are secreted phospholipase A2 molecules that inhibit transmission in neuromuscular synapses by poisoning the motor neurons. These toxins specifically and rapidly internalise into the nerve endings of motor neurons. Ammodytoxin (Atx) is a prototype β-neurotoxin from the venom of the nose-horned viper (Vipera ammodytes ammodytes). Here, we studied the relevance of the enzymatic activity of Atx in cell internalisation and subsequent intracellular movement using transmission electron microscopy (TEM). We prepared a recombinant, enzymatically inactive mutant of Atx, Atx(D49S), labelled with gold nanoparticles (GNP), and incubated this with PC12 cells, to analyse its localisation by TEM. Atx(D49S)-GNP internalised into the cells. Inside the cells, Atx(D49S)-GNP was detected in different vesicle-like structures, cytosol, endoplasmic reticulum and mitochondria, where it was spotted in the intermembrane space and matrix. Co-localization of fluorescently labelled Atx(D49S) with mitochondria in PC12 cells by confocal fluorescence microscopy confirmed the reliability of results generated using Atx(D49S)-GNP and TEM and allowed us to conclude that the phospholipase activity of Atx is not obligatory for its cell internalisation and translocation into the mitochondrial intermembrane space and matrix.

Keywords: Vipera ammodytes ammodytes; ammodytoxin; localisation; secreted phospholipase A2; snake venom; translocation; transmission electron microscopy; β-neurotoxicity.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Gold
  • Metal Nanoparticles*
  • Mitochondria
  • Neurotoxins / analysis
  • Phospholipases A2
  • Rats
  • Reproducibility of Results
  • Viper Venoms / chemistry
  • Viperidae*

Substances

  • Neurotoxins
  • Viper Venoms
  • Gold
  • Phospholipases A2

Grants and funding

This work and the APC were funded by the Slovenian Research Agency Programme grants, P1-0207 (to I.K.) and P3-0108 (to P.V.), and the Young Researcher grant 1000-17-0106-6 (to A.I.).