Structure of the active Gi-coupled human lysophosphatidic acid receptor 1 complexed with a potent agonist

Nat Commun. 2022 Sep 15;13(1):5417. doi: 10.1038/s41467-022-33121-2.

Abstract

Lysophosphatidic acid receptor 1 (LPA1) is one of the six G protein-coupled receptors activated by the bioactive lipid, lysophosphatidic acid (LPA). LPA1 is a drug target for various diseases, including cancer, inflammation, and neuropathic pain. Notably, LPA1 agonists have potential therapeutic value for obesity and urinary incontinence. Here, we report a cryo-electron microscopy structure of the active human LPA1-Gi complex bound to ONO-0740556, an LPA analog with more potent activity against LPA1. Our structure elucidated the details of the agonist binding mode and receptor activation mechanism mediated by rearrangements of transmembrane segment 7 and the central hydrophobic core. A structural comparison of LPA1 and other phylogenetically-related lipid-sensing GPCRs identified the structural determinants for lipid preference of LPA1. Moreover, we characterized the structural polymorphisms at the receptor-G-protein interface, which potentially reflect the G-protein dissociation process. Our study provides insights into the detailed mechanism of LPA1 binding to agonists and paves the way toward the design of drug-like agonists targeting LPA1.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Cryoelectron Microscopy
  • GTP-Binding Protein alpha Subunits, Gi-Go / metabolism*
  • Humans
  • Neuralgia*
  • Receptors, Lysophosphatidic Acid* / metabolism

Substances

  • Receptors, Lysophosphatidic Acid
  • GTP-Binding Protein alpha Subunits, Gi-Go