Engineering a precise adenine base editor with minimal bystander editing

Nat Chem Biol. 2023 Jan;19(1):101-110. doi: 10.1038/s41589-022-01163-8. Epub 2022 Oct 13.

Abstract

Adenine base editors (ABEs) catalyze A-to-G transitions showing broad applications, but their bystander mutations and off-target editing effects raise safety concerns. Through structure-guided engineering, we found ABE8e with an N108Q mutation reduced both adenine and cytosine bystander editing, and introduction of an additional L145T mutation (ABE9), further refined the editing window to 1-2 nucleotides with eliminated cytosine editing. Importantly, ABE9 induced very minimal RNA and undetectable Cas9-independent DNA off-target effects, which mainly installed desired single A-to-G conversion in mouse and rat embryos to efficiently generate disease models. Moreover, ABE9 accurately edited the A5 position of the protospacer sequence in pathogenic homopolymeric adenosine sites (up to 342.5-fold precision over ABE8e) and was further confirmed through a library of guide RNA-target sequence pairs. Owing to the minimized editing window, ABE9 could further broaden the targeting scope for precise correction of pathogenic single-nucleotide variants when fused to Cas9 variants with expanded protospacer adjacent motif compatibility. bpNLS, bipartite nuclear localization signals.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Adenine*
  • Animals
  • CRISPR-Cas Systems / genetics
  • Cytosine
  • Gene Editing*
  • Mice
  • Mutation
  • RNA, Guide, CRISPR-Cas Systems
  • Rats

Substances

  • Adenine
  • Cytosine
  • RNA, Guide, CRISPR-Cas Systems