Total Synthesis of Kopsone

Org Lett. 2023 Apr 21;25(15):2718-2721. doi: 10.1021/acs.orglett.3c00838. Epub 2023 Apr 10.

Abstract

A total synthesis of kopsone was achieved, featuring stereoselective preparation of an acyclic aldehyde having a protected hydroxylamine moiety via Ireland-Claisen rearrangement and intramolecular cycloaddition of an eight-membered cyclic nitrone to form the 2-azabicyclo[3.3.1]nonane skeleton.