Superior Photoprotection of Cyanine Dyes with Thio-imidazole Amino Acids

J Am Chem Soc. 2023 Sep 13;145(36):19571-19577. doi: 10.1021/jacs.3c03058. Epub 2023 Sep 1.

Abstract

Preventing fluorophore photobleaching and unwanted blinking is crucial for single-molecule fluorescence (SMF) studies. Reductants achieve photoprotection via quenching excited triplet states, yet either require counteragents or, for popular alkyl-thiols, are limited to cyanine dye Cy3 protection. Here, we provide mechanistic and imaging results showing that the naturally occurring amino acid ergothioneine and its analogue dramatically enhance photostability for Cy3, Cy5, and their conformationally restrained congeners, providing a biocompatible universal solution for demanding fluorescence imaging.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, N.I.H., Intramural

MeSH terms

  • Amino Acids
  • Ergothioneine*
  • Fluorescent Dyes
  • Imidazoles
  • Ionophores
  • Quinolines*

Substances

  • Amino Acids
  • Fluorescent Dyes
  • Imidazoles
  • Ergothioneine
  • Ionophores
  • Quinolines

Grants and funding