Propitious catalytic response of immobilized α-amylase from G. thermoleovorans in modified APTES-Fe3O4 NPs for industrial bio-processing

Int J Biol Macromol. 2024 Jun;269(Pt 1):132021. doi: 10.1016/j.ijbiomac.2024.132021. Epub 2024 Apr 30.

Abstract

Challenges in enzyme and product recovery are currently intriguing in modern biotechnology. Coping enzyme stability, shelf life and efficiency, nanomaterials-based immobilization were epitomized of industrial practice. Herein, a α-amylase from Geobacillus thermoleovorans was purified and bound effectively on to a modified 3-Aminopropyltriethoxysilane (APTES)-Fe3O4 nanoparticle. It was revealed that the carrier-bound enzyme catalysis (pH 8 and 60 °C) was significant in contrast to the free enzyme (pH 7.5 and 55 °C). Furthermore, Zn2+ and Cu2+ were shown to cause inhibitory effects in both enzyme states. Unlike chloroform, toluene, benzene, and butanol, minimal effects were observed with ethanol, acetone, and hexane. The bound enzyme retained 27.4 % of its initial activity after being stored for 36 days. In addition, the reusability of the bound enzyme showed a gradual decline in activity after the first cycle; however, after 13 cycles, its residual activity at 53 % was observed. These data proved significant enough to use this enzyme for industrial starch and analogous substrate bio-processing.

Keywords: APTES-Fe(3)O(4); FTIR; G. thermoleovorans; X-ray diffraction; α-Amylase.

MeSH terms

  • Biocatalysis
  • Catalysis
  • Enzyme Stability*
  • Enzymes, Immobilized* / chemistry
  • Enzymes, Immobilized* / metabolism
  • Geobacillus / enzymology
  • Hydrogen-Ion Concentration
  • Magnetite Nanoparticles / chemistry
  • Propylamines* / chemistry
  • Silanes / chemistry
  • Starch / chemistry
  • Temperature
  • alpha-Amylases* / chemistry
  • alpha-Amylases* / metabolism

Substances

  • Enzymes, Immobilized
  • alpha-Amylases
  • Propylamines
  • amino-propyl-triethoxysilane
  • Silanes
  • Magnetite Nanoparticles
  • Starch