Decrypting lysine deacetylase inhibitor action and protein modifications by dose-resolved proteomics

Cell Rep. 2024 Jun 25;43(6):114272. doi: 10.1016/j.celrep.2024.114272. Epub 2024 May 24.

Abstract

Lysine deacetylase inhibitors (KDACis) are approved drugs for cutaneous T cell lymphoma (CTCL), peripheral T cell lymphoma (PTCL), and multiple myeloma, but many aspects of their cellular mechanism of action (MoA) and substantial toxicity are not well understood. To shed more light on how KDACis elicit cellular responses, we systematically measured dose-dependent changes in acetylation, phosphorylation, and protein expression in response to 21 clinical and pre-clinical KDACis. The resulting 862,000 dose-response curves revealed, for instance, limited cellular specificity of histone deacetylase (HDAC) 1, 2, 3, and 6 inhibitors; strong cross-talk between acetylation and phosphorylation pathways; localization of most drug-responsive acetylation sites to intrinsically disordered regions (IDRs); an underappreciated role of acetylation in protein structure; and a shift in EP300 protein abundance between the cytoplasm and the nucleus. This comprehensive dataset serves as a resource for the investigation of the molecular mechanisms underlying KDACi action in cells and can be interactively explored online in ProteomicsDB.

Keywords: CP: Molecular biology; HDACs; acetylation; chemical proteomics; lysine deacetylase inhibitors; mass spectrometry; phosphorylation; proteomic pharmacology.

MeSH terms

  • Acetylation / drug effects
  • Cell Line, Tumor
  • Dose-Response Relationship, Drug
  • E1A-Associated p300 Protein / metabolism
  • Histone Deacetylase Inhibitors* / pharmacology
  • Histone Deacetylases / metabolism
  • Humans
  • Lysine / metabolism
  • Phosphorylation / drug effects
  • Protein Processing, Post-Translational / drug effects
  • Proteomics* / methods

Substances

  • Histone Deacetylase Inhibitors
  • Lysine
  • E1A-Associated p300 Protein
  • Histone Deacetylases