Fabrication and characterization of magnetic mesoporous nanoparticles for efficient determination and magnetic separation of sulfonamides in food samples

Anal Methods. 2024 Jun 6;16(22):3587-3596. doi: 10.1039/d4ay00590b.

Abstract

A magnetic, mesoporous core/shell structured Fe3O4@SiO2@mSiO2 nanocomposite was synthesized and employed as a magnetic solid phase extraction (MSPE) sorbent for the determination of trace sulfonamides (SAs) in food samples. The synthesized nanocomposite was characterized by transmission electron microscopy, Fourier transform infrared spectroscopy, X-ray photoelectron spectroscopy, thermogravimetric analysis, X-ray diffraction, N2 sorption analysis and vibrating sample magnetometry. The results showed that Fe3O4@SiO2@mSiO2 possessed a mesoporous structure with a large surface area. Batch experiments were carried out to investigate the adsorption ability for SAs. Fe3O4@SiO2@mSiO2 showed fast kinetics and high adsorption capacity, and the pseudo-second-order model and Langmuir adsorption isotherm are well fitted with the experimental data, indicating that chemical adsorption might be the rate-limiting step. Moreover, the high adsorption capacity can be maintained for at least 8 runs, indicating excellent stability and reusability. The proposed method exhibited good linearity in the range of 0.2-500 μg L-1, the R2 values of all the analytes were greater than 0.99 and the LODs were all lower than 0.2 μg L-1. Furthermore, real food samples were successfully analyzed with Fe3O4@SiO2@mSiO2 and high recoveries varying from 89.7% and 110.6% were obtained with low relative standard deviations ranging from 1.78% to 6.91%. The Fe3O4@SiO2@mSiO2 magnetic nanocomposite is a promising sorbent for the efficient extraction of SAs from complex food samples.

MeSH terms

  • Adsorption
  • Food Analysis / methods
  • Food Contamination / analysis
  • Limit of Detection
  • Magnetite Nanoparticles* / chemistry
  • Nanocomposites / chemistry
  • Porosity
  • Silicon Dioxide* / chemistry
  • Solid Phase Extraction* / methods
  • Sulfonamides* / analysis
  • Sulfonamides* / chemistry
  • Sulfonamides* / isolation & purification

Substances

  • Sulfonamides
  • Magnetite Nanoparticles
  • Silicon Dioxide