Nicardipine-chitosan nanoparticles alleviate thioacetamide-induced acute liver injury by targeting NFκB/NLRP3/IL-1β signaling in rats: Unraveling new roles beyond calcium channel blocking

Int Immunopharmacol. 2024 Nov 15:141:113000. doi: 10.1016/j.intimp.2024.113000. Epub 2024 Aug 27.

Abstract

Liver inflammatory diseases are marked by serious complications. Notably, nicardipine (NCD) has demonstrated anti-inflammatory properties, but its benefits in liver inflammation have not been studied yet. However, the therapeutic efficacy of NCD is limited by its short half-life and low bioavailability. Therefore, we aimed to evaluate the potential of NCD-loaded chitosan nanoparticles (ChNPs) to improve its pharmacokinetic profile and hepatic accumulation. Four formulations of NCD-ChNPs were synthesized and characterized. The optimal formulation (NP2) exhibited a mean particle diameter of 172.6 ± 1.94 nm, a surface charge of +25.66 ± 0.93 mV, and an encapsulation efficiency of 88.86 ± 1.17 %. NP2 showed good physical stability as a lyophilized powder over three months. It displayed pH-sensitive release characteristics, releasing 77.15 ± 5.09 % of NCD at pH 6 (mimicking the inflammatory microenvironment) and 52.15 ± 3.65 % at pH 7.4, indicating targeted release in inflamed liver tissues. Pharmacokinetic and biodistribution studies revealed that NCD-ChNPs significantly prolonged NCD circulation time and enhanced its concentration in liver tissues compared to plain NCD. Additionally, the study investigated the protective effects of NCD-ChNPs in thioacetamide-induced liver injury in rats by modulating the NFκB/NLRP3/IL-1β signaling axis. NCD-ChNPs effectively inhibited NFκB activation, reduced NLRP3 inflammasome activation, and subsequent release of IL-1β, which correlated with improved hepatic function and reduced inflammation and oxidative stress. These findings highlight the potential of NCD-ChNPs as a promising nanomedicine strategy for the treatment of liver inflammatory diseases, warranting further investigation into their clinical applications, particularly in hypertensive patients with liver inflammatory conditions.

Keywords: Chitosan nanoparticles; Liver biodistribution; Liver inflammatory diseases; NFκB/NLRP3/IL-1β signaling; New therapeutic target; Nicardipine.

MeSH terms

  • Animals
  • Anti-Inflammatory Agents / pharmacology
  • Anti-Inflammatory Agents / therapeutic use
  • Calcium Channel Blockers / administration & dosage
  • Calcium Channel Blockers / pharmacology
  • Calcium Channel Blockers / therapeutic use
  • Chemical and Drug Induced Liver Injury* / drug therapy
  • Chitosan* / chemistry
  • Interleukin-1beta* / metabolism
  • Liver / drug effects
  • Liver / metabolism
  • Liver / pathology
  • Male
  • NF-kappa B* / metabolism
  • NLR Family, Pyrin Domain-Containing 3 Protein* / metabolism
  • Nanoparticles* / chemistry
  • Nicardipine* / administration & dosage
  • Nicardipine* / pharmacology
  • Nicardipine* / therapeutic use
  • Rats
  • Rats, Sprague-Dawley
  • Signal Transduction* / drug effects
  • Thioacetamide*
  • Tissue Distribution

Substances

  • Chitosan
  • NLR Family, Pyrin Domain-Containing 3 Protein
  • NF-kappa B
  • Nlrp3 protein, rat
  • Interleukin-1beta
  • Thioacetamide
  • Nicardipine
  • Calcium Channel Blockers
  • Anti-Inflammatory Agents
  • IL1B protein, rat