Mammalian Esterase Activity: Implications for Peptide Prodrugs

Biochemistry. 2024 Oct 15;63(20):2580-2593. doi: 10.1021/acs.biochem.4c00446. Epub 2024 Oct 3.

Abstract

As a traceless, bioreversible modification, the esterification of carboxyl groups in peptides and proteins has the potential to increase their clinical utility. An impediment is the lack of strategies to quantify esterase-catalyzed hydrolysis rates for esters in esterified biologics. We have developed a continuous Förster resonance energy transfer (FRET) assay for esterase activity based on a peptidic substrate and a protease, Glu-C, that cleaves a glutamyl peptide bond only if the glutamyl side chain is a free acid. Using pig liver esterase (PLE) and human carboxylesterases, we validated the assay with substrates containing simple esters (e.g., ethyl) and esters designed to be released by self-immolation upon quinone methide elimination. We found that simple esters were not cleaved by esterases, likely for steric reasons. To account for the relatively low rate of quinone methide elimination, we extended the mathematics of the traditional Michaelis-Menten model to conclude with a first-order intermediate decay step. By exploring two regimes of our substrate → intermediate → product (SIP) model, we evaluated the rate constants for the PLE-catalyzed cleavage of an ester on a glutamyl side chain (kcat/KM = 1.63 × 103 M-1 s-1) and subsequent spontaneous quinone methide elimination to regenerate the unmodified peptide (kI = 0.00325 s-1; t1/2 = 3.55 min). The detection of esterase activity was also feasible in the human intestinal S9 fraction. Our assay and SIP model increase the understanding of the release kinetics of esterified biologics and facilitate the rational design of efficacious peptide prodrugs.

Publication types

  • Research Support, N.I.H., Extramural

MeSH terms

  • Animals
  • Esterases* / chemistry
  • Esterases* / metabolism
  • Esters / chemistry
  • Esters / metabolism
  • Fluorescence Resonance Energy Transfer
  • Humans
  • Hydrolysis
  • Kinetics
  • Liver / enzymology
  • Peptides* / chemistry
  • Peptides* / metabolism
  • Prodrugs* / chemistry
  • Prodrugs* / metabolism
  • Substrate Specificity
  • Swine

Substances

  • Prodrugs
  • Peptides
  • Esterases
  • Esters