Characterization of Phytoplankton-Derived Amino Acids and Tracing the Source of Organic Carbon Using Stable Isotopes in the Amundsen Sea

Mar Drugs. 2024 Oct 18;22(10):476. doi: 10.3390/md22100476.

Abstract

We utilized amino acid (AA) and carbon stable isotope analyses to characterize phytoplankton-derived organic matter (OM) and trace the sources of organic carbon in the Amundsen Sea. Carbon isotope ratios of particulate organic carbon (δ13C-POC) range from -28.7‱ to -23.1‱, indicating that particulate organic matter originated primarily from phytoplankton. The dissolved organic carbon isotope (δ13C-DOC) signature (-27.1 to -21.0‱) observed in the sea-ice melting system suggests that meltwater contributes to the DOC supply of the Amundsen Sea together with OM produced by phytoplankton. A negative correlation between the degradation index and δ13C-POC indicates that the quality of OM significantly influences isotopic fractionation (r2 = 0.59, p < 0.001). The AA distribution in the Amundsen Sea (5.43 ± 3.19 µM) was significantly larger than previously reported in the Southern Ocean and was associated with phytoplankton biomass (r2 = 0.49, p < 0.01). Under conditions dominated by P. antarctica (DI = 2.29 ± 2.30), OM exhibited greater lability compared to conditions co-dominated by diatoms and D. speculum (DI = 0.04 ± 3.64). These results highlight the important role of P. antarctica in influencing the properties of OM, suggesting potential impacts on carbon cycling and microbial metabolic activity in the Amundsen Sea.

Keywords: Amundsen Sea; P. antarctica; amino acid; antarctica; stable isotope.

MeSH terms

  • Amino Acids* / analysis
  • Amino Acids* / metabolism
  • Biomass
  • Carbon Isotopes* / analysis
  • Carbon* / metabolism
  • Diatoms / metabolism
  • Oceans and Seas
  • Phytoplankton* / metabolism
  • Seawater / chemistry

Substances

  • Carbon Isotopes
  • Amino Acids
  • Carbon

Grants and funding

This research was supported by the Korea Polar Research Institute (KOPRI, PE24110) and the National Institute of Environmental Research (NIER, 2024-01-01-055).