Spectrally Tunable Ultrafast Long Wave Infrared Detection at Room Temperature

Nano Lett. 2024 Nov 20;24(46):14678-14685. doi: 10.1021/acs.nanolett.4c03832. Epub 2024 Nov 6.

Abstract

Room-temperature longwave infrared (LWIR) detectors are preferred over cryogenically cooled solutions due to the cost effectiveness and ease of operation. The performance of present uncooled LWIR detectors such as microbolometers, is limited by reduced sensitivity, slow response time, and the lack of dynamic spectral tunability. Here, we present a graphene-based efficient room-temperature LWIR detector with high detectivity and fast response time utilizing its tunable optical and electronic characteristics. The inherent weak light absorption is enhanced by Dirac plasmons on the patterned graphene coupled to an optical cavity. The absorbed energy is converted into photovoltage by the Seebeck effect with an asymmetric carrier generation environment. Further, dynamic spectral tunability in the 8-12 μm LWIR band is achieved by electrostatic gating. The proposed detection platform paves the path to a fresh generation of uncooled graphene-based LWIR photodetectors for wide ranging applications such as molecular sensing, medical diagnostics, military, security and space.

Keywords: Dirac plasmons; graphene; infrared detector; photothermoelectric effect; two-dimensional materials.