Synthesis of anisotropic Janus composite particles based on polystyrene/urushiol- lanthanum chelate polymer

PLoS One. 2024 Dec 3;19(12):e0314449. doi: 10.1371/journal.pone.0314449. eCollection 2024.

Abstract

To expand the potential applications of raw lacquer, snowman-like polystyrene (PS)-urushiol lanthanum (ULa) Janus composite particles were synthesized by emulsion swelling-assisted protrusion from PS/ULa core-shell composite microspheres. The morphology and chemical composition of the PS/ULa composite microspheres and the PS-ULa Janus composite particles were investigated with scanning electron microscopy (SEM), transmission electron microscopy (TEM), energy dispersive X-ray (EDX), thermogravimetric analysis (TGA), and Fourier transform infrared (FT-IR). The PS-ULa Janus particles were compartmentalized into two parts, each with a different morphology and chemical composition. Results showed that the intact ULa shell with appropriate thickness is a crucial factor for controllable swelling, and the thickness of the PS/ULa core-shell composite microsphere could be controlled by polymerization temperature. This anisotropic Janus particle exhibits potential applications in orienting materials, such as directional catalysis.

MeSH terms

  • Anisotropy
  • Chelating Agents / chemical synthesis
  • Chelating Agents / chemistry
  • Lanthanum* / chemistry
  • Microscopy, Electron, Scanning
  • Microscopy, Electron, Transmission
  • Microspheres
  • Particle Size
  • Polymers / chemistry
  • Polystyrenes* / chemistry
  • Spectroscopy, Fourier Transform Infrared
  • Thermogravimetry

Substances

  • Polystyrenes
  • Lanthanum
  • Polymers
  • Chelating Agents

Grants and funding

This work was funded by Natural Science Foundation of Fujian Province (Grant No. 2023J011798) and Foundation of Fujian Educational Committee (Grant No. JAT220680) to YZ. The funders played no role in the study design, data collection and analysis, decision to publish, or preparation of the manuscript.