Susceptibility of gamma-irradiated proteins to in vitro glycation: exposure to oxygen free radicals increases glycation-induced modifications

Cell Biochem Funct. 1996 Jun;14(2):149-54. doi: 10.1002/cbf.658.

Abstract

Oxidation and glycation are non-enzymatic protein modifications involved in the pathogenesis of aging. We evaluated their possible influences in an in vitro system: albumin was oxidized by gamma-irradiation and then exposed to glycation in vitro. Fluorescence modifications were analysed as signals of protein alterations. Both radiolytic oxidation and in vitro glycation provoked a sharp decrease of tryptophan fluorescence (278 nm ex./340 nm em.); their effects tended to be additive, unless a saturation limit was reached. Both individually and in combination, these two non-enzymatic processes induced the appearance of a new fluorescence (335 nm ex./415 nm em.); in this case as well there was an additive effect, with a trend toward saturation. Radiolytic oxidation and in vitro glycation seem to provoke similar damage to the exposed proteins: the observed fluorescence alterations may be due to similar conformational changes, breaks or the development of fluorophores.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Aging / metabolism
  • Dose-Response Relationship, Radiation
  • Fluorescent Dyes
  • Free Radicals / chemistry
  • Free Radicals / metabolism
  • Gamma Rays
  • Glucose / chemistry
  • Glucose / metabolism
  • Glycosylation
  • Oxidation-Reduction
  • Protein Conformation
  • Reactive Oxygen Species / chemistry
  • Reactive Oxygen Species / metabolism*
  • Serum Albumin, Bovine / chemistry
  • Serum Albumin, Bovine / metabolism*
  • Serum Albumin, Bovine / radiation effects*
  • Tryptophan / chemistry
  • Tryptophan / radiation effects

Substances

  • Fluorescent Dyes
  • Free Radicals
  • Reactive Oxygen Species
  • Serum Albumin, Bovine
  • Tryptophan
  • Glucose