Identification of the catalytic nucleophile of endoglucanase I from Fusarium oxysporum by mass spectrometry

Biochemistry. 1997 May 13;36(19):5893-901. doi: 10.1021/bi962962h.

Abstract

The endoglucanase EG I from Fusarium oxysporum catalyzes the hydrolysis of cellulose via a double-displacement mechanism involving the formation and hydrolysis of a glycosyl-enzyme intermediate. Treatment of EG I with 2',4'-dinitrophenyl-2-deoxy-2-fluoro-beta-D-cellobioside results in the time-dependent inactivation of the enzyme (k(i) = 1.36 min(-1), Ki = 0.88 mM) via trapping of a covalent 2-deoxy-2-fluorocellobiosyl-enzyme intermediate. This intermediate is, however, catalytically competent undergoing transglycosylation, thus reactivation, in the presence of D-cellobiose. Analysis of a peptic digest of the inactivated enzyme by HPLC/ESMS/MS in the neutral loss mode allowed identification of a 2-fluorocellobiosyl-labeled peptide containing Glu197. This was confirmed by comparative mapping studies and subsequent Edman degradation analysis. This residue is completely conserved in glycosidase family 7, to which EG I belongs, consistent with its key role as the catalytic nucleophile.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Binding Sites
  • Catalysis
  • Cellulase / metabolism*
  • Cellulose 1,4-beta-Cellobiosidase
  • Enzyme Activation
  • Fungal Proteins / metabolism*
  • Glutamic Acid / metabolism
  • Kinetics
  • Mass Spectrometry
  • Molecular Sequence Data
  • Peptides / metabolism

Substances

  • Fungal Proteins
  • Peptides
  • Glutamic Acid
  • Cellulase
  • Cellulose 1,4-beta-Cellobiosidase