Construction and characterization of an OHIO-1 beta-lactamase bearing Met69Ile and Gly238Ser mutations

Antimicrob Agents Chemother. 1997 Sep;41(9):1940-3. doi: 10.1128/AAC.41.9.1940.

Abstract

Amino acid changes that influence activity and resistance to beta-lactams and beta-lactamase inhibitors were explored by constructing the Gly238Ser and Met69Ile-Gly238Ser mutants of the OHIO-1 beta-lactamase, a class A enzyme of the SHV family. The Km values of cefotaxime and ceftazidime for OHIO-1 and Met69Ile beta-lactamases were > or = 500 microM. The Km of cefotaxime for the Gly238Ser beta-lactamase was 26 microM, and that of ceftazidime was 105 microM. The Km of cefotaxime for the Met69Ile-Gly238Ser beta-lactamase was 292 microM, and that of ceftazidime was 392 microM. For the beta-lactamase inhibitors clavulanate and sulbactam, the apparent Ki values for the Met69Ile-Gly238Ser enzyme were 0.03 and 0.15 microM, respectively. Relative Vmax values indicate that the Met69Ile-Gly238Ser mutant of the OHIO-1 beta-lactamase possesses cephalosporinase activity similar to that of the Gly238Ser mutant but diminished penicillinase activity. In an Escherichia coli DH5alpha strain that possesses a Met69Ile beta-lactamase of the OHIO-1 family, the added Gly238Ser mutation resulted in a phenotype with qualities that confer resistance to expanded-spectrum cephalosporins and, to a lesser extent, beta-lactamase inhibitors.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Cephalosporin Resistance
  • Enzyme Inhibitors / pharmacology
  • Glycine / genetics
  • Glycine / metabolism
  • Isoleucine / genetics
  • Isoleucine / metabolism
  • Kinetics
  • Methionine / genetics
  • Methionine / metabolism
  • Mutagenesis, Site-Directed
  • Mutation*
  • Phenotype
  • Serine / genetics
  • Serine / metabolism
  • beta-Lactam Resistance
  • beta-Lactamases / biosynthesis
  • beta-Lactamases / genetics*
  • beta-Lactamases / metabolism*

Substances

  • Enzyme Inhibitors
  • Isoleucine
  • Serine
  • Methionine
  • beta-Lactamases
  • Glycine